Brian Rosen

 

 

 

 

 

 

Talk: Discovering the right transition metal carbide alloy for electrocatalysis 

 Catalysts used in polymer electrolyte membrane fuel cells (PEMFCs) are often supported by carbon, which is susceptible to corrosion at operating potentials. Transition metal carbides (TMCs) are a class of material that could be used as catalyst supports to replace carbon as they are electrically conductive and can be resistant to such corrosion. TMCs which show promising activity for the oxygen reduction reaction (ORR), however, have been shown to suffer from oxidation, whereas corrosion-resistant carbides tend to have significantly lower ORR activities. Here we show with computational and experimental evidence that alloying between different types of carbides can be an effective technique to meet both the activity and durability needs of fuel cells, and more broadly, electrochemical devices. We investigate the effect on both 3D and 2D transition metal carbides based on titanium and molybdenum while substituting oxyphilic atoms such as tantalum, hafnium, and niobium. Given the exceedingly large number of possible materials, computational techniques are used to guide experimental synthesis in order to narrow the field of potentially successful materials. ​ 

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